Adsorption analysis: Equilibria and kinetics by Do D.D.

By Do D.D.

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J. C. Light, Disc. , 44, 14 (1967). 9. (a) J. C. Polanyi and S. D. Rosner, J. Chem. Phys. 38, 1028 (1963); (b) P. J. Kuntz, E. M. Nerneth, J. C. Polanyi, S. D. Rosner, and C. E. Young, J. Chem. Phys. 44, 1168 (1966); (c) K. G. Anlauf, J. C. Polanyi, W. H. Wong, and K. B. Woodall, J. Chem. Phys. 49, 5189 (1968); (d) P. J. Kuntz, E. M. Nemeth, and J. C. Polanyi, J. Chem. Phys. 50, 4607 (1969); (e) P. J. Kuntz, M. H. Mok, and J. C. Polanyi, J . Chem. Phys. 50,4623 (1969). 10. (a) N. C. Blais and D.

The energy of these reactions must be disposed of as kinetic energy in the products because there are no accessible internal energy states available in the neutral helium or H + products, and H atoms do not appear to be a suitable energy sink for the amount of energy that has to be dissipated. The conversion of internal to kinetic energy was shown again to be a process requiring very small impact parameter collisions. The single source work on low energy elemental ion reactions which gave experimental results in very good agreement with G-S theory was not initially accepted without reservation because of difficulties encountered by many workers in their attempts to carry out single source experiments.

A) M. Karplus, R. N. Porter, and R. D. Sharma, J. Chem. Phys. 40, 2033 (1964); 43, 3259 (1965); (b) M. Godfrey and M. Karplus, J . Chem. Phys. 49, 3602 (1968). 12. M. G. Evans and M. Polanyi, Trans. 35, 178 (1939). QUANTUM THEORIES OF CHEMICAL KINETICS 31 13. D. J. Kouri, J. Chem. Phys. 51, 5204 (1969). 14. W. N. Sams and D. J. Kouri, J. Chem. Phys. 51,4809 (1969). 15. D. Micha, Arkiv. For Fysik 30, 425 (1965). 16. M. Karplus and K. T. Faraday Soc. 44, 56 (1967). 17. H. Hulbert and J . Hirschfelder, J .

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